Transport phenomena and microscopic structure in partially miscible binary fluids: A simulation study of the symmetrical Lennard-Jones mixture

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Transport phenomena and microscopic structure in partially miscible binary fluids: A simulation study of the symmetrical Lennard-Jones mixture

Static and dynamic structure factors and various transport coefficients are computed for a Lennard-Jones model of a binary fluid (A,B) with a symmetrical miscibility gap, varying both temperature and relative concentration of the mixture. The model is first equilibrated by a semi-grandcanonical Monte Carlo method, choosing the temperature and chemical potential difference ∆μ between the two spe...

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Abstract A Lennard–Jones model of a binary dense liquid (A,B) with a symmetrical miscibility gap is investigated by means of computer simulation methods. Semigrand–canonical Monte Carlo simulations yield the phase diagram in the T–x plane (T : temperature, x: concentration of A or B particles) as well as equilibrated configurations at coexistence. Then Molecular Dynamics simulations use these c...

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ژورنال

عنوان ژورنال: The Journal of Chemical Physics

سال: 2003

ISSN: 0021-9606,1089-7690

DOI: 10.1063/1.1580106